I don't think you have any idea how complex what you're proposing is.
So complex that similar operations were performed by BR works on numerous occasions, sometimes for periods of only months in operation?
See fitting on TDM gear to Class 43s, fitting various locomotives with Mark 1 EMU control systems and so on and so on.
There's a serious issue building new diesel locos for the UK, as there's no current design that fits the UK loading gauge and complies with current emissions legislation. There was a limit on the number of Class 68s allowed to be built, and no more are permitted.
Well if we really cant build new locomotives then I think railfreight is even more stuffed than I thought it was.....
Locomotives are also incredibly expensive compared to the cost of multiple unit vehicles.
They are more expensive yes, but most information I see suggests two or three times the price, rather than eight times.......
So the capital cost is still much lower than procuring eight car multiple unit sets from scratch.
What you're proposing also involves having to mash up potentially massively incompatible control systems and possibly make extensive alterations to the MUs involved.
The MUs in question have no major TMS style electronic control systems, and as has been repeatedly demonstrated in the US (where essentially all locomotives, including those built by a large number of disparate manufacturers, can be operated in multiple, making systems work with non electronic control systems is relatively simple)
If locomotive builders can make their fancy control systems work with an ancient AAR control standard, they can make it work with a non-electronic electrical control system like that fitted to Mark 3 EMUs.
It wouldn't even be a small job as the RSSB gives essentially the same MU control gear for all the Mark 3 EMUs and the Networkers.
Which means potentially hundreds of eight-car sets.
The only reason locomotives and multiple units are built with proprietary TMS systems is to ensure manufacturer lock in.